Nucleation


The scope of my interests now concerns the investigation of the initial stages of nucleation in minerals by low-frequency Raman
and Fourier transform spectroscopies. Our preliminary results show that these methods are highly effective for studying the structure micro-inhomogeneities of the size from 1 to 10 nm. It should be noted, that the initial stages of nucleation, are detected by Raman scattering, when the infrared spectroscopy, and the X-ray diffraction, do not show any change. We have investigated of the influence of the structural disorder in the amorphous solids, which came before the nucleation, on the intensity of light scattering by the acoustic phonons. We have observed experimentally [NN Ovsyuk and VN Novikov. Phys. Rev. B 57, 14615 (1998)] that in the low-frequency Raman light scattering spectrum of the amorphous solids the boson peak situated in the acoustic range is more sensitive to the structural order than the optical mode presently used to determine the degree of disorder. We have shown that this is because, unlike the coefficient of interaction with optical vibrations, the coefficient of interaction between light and acoustic vibrations contains an additional factor, the square of the reciprocal correlation length of the vibrational excitations, i.e., the intensity of light scattering by acoustic phonons has an additional dependence on the degree of disorder. Thus, the results of our studies, have shown, that the low-frequency Raman scattering, allow us, to observe modifications of the correlation length, at early stages of crystallization. For our studies, we took silicon and germanium, as well known models. The regularities obtained, will be valid for minerals also.
The low-frequency Raman scattering appears to be a sensitive method for the investigation of the initial stage of nucleation in multi-
and monocomponent systems [NN Ovsyuk. Europhys. Lett. 89, 26001 (2010)]. In the case of the mono-component systems, when the crystalline nuclei do not have an acoustic mismatch as compared to the amorphous matrix, we cannot observe their surface vibrations, but we can make use of the fact that in nucleation there is a jump in a structure correlation length. This results in a sharp decrease in contribution to the density of the acoustic vibration states because of decreasing the concentration of structural correlations on which acoustic phonons are localized. In addition, low-frequency Raman spectroscopy may be useful in the research into the phase transformation in materials for phase-change memories.